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K. H. Kang

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Visualization of flow inside a small evaporating droplet

 

Kwan Hyoung Kang, Sang Joon Lee, Choung Mook Lee, and In Seok Kang

Department of Mechanical Engineering, Pohang University of Science and Technology, San 31, Hyoja-dong, Pohang 790-784, Republic of Korea

(Selected for publication in the special issue of the Measurement Science & Technology

for PIV¡¯03)

 

Droplets have many interesting applications associated with microfluidic problems, e.g., DNA molecules imaging, micro-pumps, and ink-jet printing. The details of droplet-related phenomena in micro and nanoscales such as evaporation process, Marangoni effects, contact angles with solid substrates, and electrowetting are not well known. There is a consensus of opinion that the fluid flow inside a droplet may play an important role on the overall transport phenomena. Compared to its importance of fluid flows, only a few systematic investigations have been performed in the past, toward understanding of overall transport phenomena inside a droplet.

 

 

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Fig. 1. Verification of the image-restoring method. (a) Plexiglas lens; (b) original image; (c) restored image. The accuracy of the present image restoration method which incorporates the ray-tracing method is checked by using a hemi-spherical Plexiglas lens (see Fig. 1a). In Fig. 1b, the distorted image of 30¡¿15 meshes due to the presence of the hemi-spherical Plexiglas lens is shown. The restored image by using the ray-tracing method is shown in Fig. 1c. The center region is well restored, while the accuracy of image restoration is not so good for the region of r/Ro > 0.75.

          

 

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Fig. 2 Flow inside evaporating droplets for different concentration of ethanol at 20 sec exposure except for (d) at 2 sec exposure. (a) 1%; (b) 5%; (c) 20%; (d) 20%. The flow is upward at the center region for all the cases. For the case of 5% mixture, the flow is initially rather unstable at the periphery of the droplet as shown in Fig. 2b. In all the cases considered here, the regular flow patterns such as shown in Figs. 2a and 2c are established after moderate times. A similar flow pattern is also observed when KCl (sodium chloride) mixed with deionized water is used. It is very intriguing phenomenon that very small amount of additives generates such a change in the fluid motion. It is conjectured that the flow shown in Fig. 2 is either driven by the density gradient inside a droplet or by viscous diffusion, rather than by the Marangoni instability.

 

 

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Fig. 3 Restoration of velocity vectors for the case of 1% mixture. (a) before restoration; (b) after restoration. The most important difference between the two results is that the magnitude of upward velocity component at the center region of the droplet is reduced after the image restoration. Additionally, the center of vorticity is moved a little towards the origin.

 


Lastly Modified in October 13, 2003